Direct bus options from San Antonio, TX to Monterrey, NL Mexico?

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Essentially, no. Bear in mind border crossings may require a change of bus, or at the least, a delay while an entire bus goes through passport control. That takes a lot longer than one car load, so it's not entirely fair to compare the two.

Rome2Rio shows 3 options for bus, ranging from 6h47 to 11h21.

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